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Springer Theses

Chemistry in Action: Making Molecular Movies with Ultrafast Electron Diffraction and Data Science

Authors: Liu, Lai Chung

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  • Nominated as an outstanding PhD thesis by the University of Toronto
  • Includes an accessible introduction to transient absorption spectroscopy, ultrafast electron diffraction, and related data science techniques
  • Describes a groundbreaking process for the direct observation of atoms and molecules undergoing chemical reactions
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書籍の購入

イーブック ¥16,015
価格の適用国: Japan (日本円価格は個人のお客様のみ有効) (小計)
  • ISBN 978-3-030-54851-3
  • ウォーターマーク付、 DRMフリー
  • ファイル形式: PDF, EPUB
  • ebooks can be used on all reading devices
  • Immediate eBook download after purchase
ハードカバー ¥20,019
価格の適用国: Japan (日本円価格は個人のお客様のみ有効) (小計)
この書籍について

The thesis provides the necessary experimental and analytical tools to unambiguously observe the atomically resolved chemical reactions. A great challenge of modern science has been to directly observe atomic motions during structural transitions, and while this was first achieved through a major advance in electron source brightness, the information content was still limited and new methods for image reconstruction using femtosecond electron diffraction methods were needed. One particular challenge lay in reconciling the innumerable possible nuclear configurations with the observation of chemical reaction mechanisms that reproducibly give the same kind of chemistry for large classes of molecules. The author shows that there is a simple solution that occurs during barrier crossing in which the highly anharmonic potential at that point in nuclear rearrangements couples high- and low-frequency vibrational modes to give highly localized nuclear motions, reducing hundreds of potential degrees of freedom to just a few key modes. Specific examples are given in this thesis, including two photoinduced phase transitions in an organic system, a ring closure reaction, and two direct observations of nuclear reorganization driven by spin transitions. The emerging field of structural dynamics promises to change the way we think about the physics of chemistry and this thesis provides tools to make it happen.

著者について

Dr. Lai Chung Liu received his PhD from the University of Toronto in 2019.

Table of contents (7 chapters)

Table of contents (7 chapters)

書籍の購入

イーブック ¥16,015
価格の適用国: Japan (日本円価格は個人のお客様のみ有効) (小計)
  • ISBN 978-3-030-54851-3
  • ウォーターマーク付、 DRMフリー
  • ファイル形式: PDF, EPUB
  • ebooks can be used on all reading devices
  • Immediate eBook download after purchase
ハードカバー ¥20,019
価格の適用国: Japan (日本円価格は個人のお客様のみ有効) (小計)
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書誌情報

Bibliographic Information
Book Title
Chemistry in Action: Making Molecular Movies with Ultrafast Electron Diffraction and Data Science
Authors
Series Title
Springer Theses
Copyright
2020
Publisher
Springer International Publishing
Copyright Holder
Springer Nature Switzerland AG
イーブック ISBN
978-3-030-54851-3
DOI
10.1007/978-3-030-54851-3
ハードカバー ISBN
978-3-030-54850-6
Series ISSN
2190-5053
Edition Number
1
Number of Pages
XX, 239
Number of Illustrations
4 b/w illustrations, 106 illustrations in colour
Topics