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Coherent Multidimensional Spectroscopy

  • Book
  • © 2019

Overview

Editors:
  1. Minhaeng Cho

    1. Department of Chemistry, Korea University, Seoul, Korea (Republic of)

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  • Offers complete theoretical descriptions of coherent multidimensional spectroscopy (CMDS) to further understanding of the underlying principles
  • Describes applications of CMDS over a broad range of frequencies to demonstrate its versatility
  • Helps researchers and graduate students to develop novel tools in spatial and time-resolved vibrational and electronic spectroscopy and imaging

Part of the book series: Springer Series in Optical Sciences (SSOS, volume 226)

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Table of contents (16 chapters)

  1. Front Matter

    Pages i-xviii
    Download chapter PDF

  2. Introduction to Coherent Multidimensional Spectroscopy

    • Minhaeng Cho
    Pages 1-34

  3. Two-Dimensional Electronic Vibrational Spectroscopy

    • Graham R. Fleming, Nicholas H. C. Lewis, E. A. Arsenault, Eric C. Wu, Sabine Oldemeyer
    Pages 35-49

  4. Nuclear Wave-Packet Dynamics in Two-Dimensional Interferograms of Excitation-Transfer Systems

    • Jeffrey A. Cina, Alexis J. Kiessling
    Pages 51-85

  5. The Development and Applications of Phase Cycling in Multidimensional Optical Spectroscopy

    • Howe-Siang Tan
    Pages 87-103

  6. Four-Dimensional Coherent Spectroscopy

    • Elad Harel
    Pages 105-124

  7. Two-Dimensional Electronic Spectroscopy of Gold Nanorods: Nodal Line Slope Analysis and Spectral Interference

    • Hanju Rhee, Minhaeng Cho
    Pages 125-143

  8. Fully Coherent Schrodinger Cat State Spectroscopy and the Future of CMDS

    • John C. Wright
    Pages 145-170

  9. Noncovalent Interactions of Hydrated DNA and RNA Mapped by 2D-IR Spectroscopy

    • Benjamin P. Fingerhut, Thomas Elsaesser
    Pages 171-195

  10. Two-Dimensional Terahertz-Infrared-Visible Spectroscopy Elucidates Coupling Between Low- and High-Frequency Modes

    • Laura Vietze, Mischa Bonn, Maksim Grechko
    Pages 197-214

  11. Ultrafast Vibrational Dynamics at Aqueous Interfaces Studied by 2D Heterodyne-Detected Vibrational Sum Frequency Generation Spectroscopy

    • Ken-ichi Inoue, Satoshi Nihonyanagi, Tahei Tahara
    Pages 215-236

  12. Ultrafast Spectroscopy of Hydrogenase Enzyme Models

    • Peter A. Eckert, Kevin J. Kubarych
    Pages 237-258

  13. Vibrational Frequency Fluctuations of Ionic and Non-ionic Vibrational Probe Molecules in Aqueous Solutions

    • Masaki Okuda, Masahiro Higashi, Kaoru Ohta, Shinji Saito, Keisuke Tominaga
    Pages 259-285

  14. Surface-Enhanced 2DIR Spectroscopy of nm-Thick Films Using Plasmonic Nano-arrays

    • Robert T. Mackin, Bar Cohn, Lev Chuntonov, Igor V. Rubtsov
    Pages 287-310

  15. The Development of Coherent Multidimensional Microspectroscopy

    • Clara A. Tibbetts, Bradley M. Luther, Amber T. Krummel
    Pages 311-337

  16. Frequency Comb-Based Multidimensional Coherent Spectroscopy

    • Bachana Lomsadze, Steven T. Cundiff
    Pages 339-354

  17. Nonlinear Spectroscopy of Chromophores in Condensed Phases with Multiple Frequency Combs

    • JunWoo Kim, Minhaeng Cho
    Pages 355-379

  18. Back Matter

    Pages 381-394
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Keywords

About this book

This book will fulfill the needs of time-domain spectroscopists who wish to deepen their understanding of both the theoretical and experimental features of this cutting-edge spectroscopy technique. Coherent Multidimensional Spectroscopy (CMDS) is a state-of-the-art technique with applications in a variety of subjects like chemistry, molecular physics, biochemistry, biophysics, and material science. Due to dramatic advancements of ultrafast laser technologies, diverse multidimensional spectroscopic methods utilizing combinations of THz, IR, visible, UV, and X-ray radiation sources have been developed and used to study real time dynamics of small molecules in solutions, proteins and nucleic acids in condensed phases and membranes, single and multiple excitons in functional materials like semiconductors, quantum dots, and solar cells, photo-excited states in light-harvesting complexes, ions in battery electrolytes, electronic and conformational changes in charge or proton transfer systems, and excess electrons and protons in water and biological systems.

Editors and Affiliations

  • Department of Chemistry, Korea University, Seoul, Korea (Republic of)

    Minhaeng Cho

About the editor

Minhaeng Cho was born in Seoul. He received B.S. and M.S. degrees in chemistry from Seoul National University in 1987 and 1989 and a Ph.D. from University of Chicago in 1993 under the direction of Graham R. Fleming. After two years of postdoctoral training at MIT in Robert J. Silbey’s group from 1994 to 1996, he has been on the faculty of Korea University since March 1996, where he was the director of the Center for Multidimensional Spectroscopy from 2000 to 2009. In December 2014, he was appointed as the Director of the IBS (Institute for Basic Science) Center for Molecular Spectroscopy and Dynamics, located in Korea University, Seoul, South Korea.

His research interests are theoretical and computational chemistry and ultrafast nonlinear optical spectroscopy. He was elected as a member of the Korean Academy of Science and Technology (KAST) in 2002. He is a recipient of the Nobel Laureate Signatures Award (American Chemical Society) in 1995, Young Scientist Award (Ministry of Science and Technology, Korea) in 1999, Kyung-Am Prize in 2010, KAST Award in 2011, and Korea National Academy of Science Award in 2012.

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